To unpair endpoint:
Open Google Chrome browser and click Chrome Vault icon located on the toolbar.
Go to More option
icon > Admin Mode.
The Chrome Vault login screen is displayed on a new tab.
Enter your credentials to log in to admin mode.
On the home screen, select Unpair Endpoint.
The Confirm Unpair screen is displayed.
Select Confirm.
The device is unpaired successfully.
Watch our video How to unpair endpoint in Chrome Vault- Video Tutorial